Numerical Modeling and Experimental Study of Elastic-Plastic Behavior of Carbon Nanotubes Reinforced Nanocompsites of PA6/NBR Using a Microfinite Element Model

Document Type : Research Paper

Authors

Department of Rubber Processing and Engineering, Faculty of Processing, Iran Polymer and Petrochemical Institute, P.O. Box: 14975-112, Tehran, Iran

Abstract

A theoretical and experimental study was conducted on the mechanical behavior of nanocomposites based on PA6/NBR thermoplastic elastomer reinforced by single wall carbon nanotubes (SWNTs). The selected samples include 60 and 40% NBR with 0.5, 1.0 and 1.5% SWNT. The modeling methodology was based on the use of two-dimensional "representative volume elements" (RVE). The Abaqus/standard code was employed to carry out the non-linear finite element calculations. Plane stress elements were selected for discretization of the domain. Linear elastic and isotropic hardening elastic-plastic models were utilized to describe the mechanical behaviors of the carbon nanotubes and polymer matrix, respectively. The samples were simultaneously prepared using melt mixing method in a laboratory internal mixer. Different orientations including regular in both longitudinal and transverse directions and random were selected for the nanotubes in the matrix. Also, two structural forms including hollow and solid for the carbon nanotubes were chosen. The highest and lowest predicted moduli were obtained from models with regular orientation in longitudinal and transverse directions, respectively. On the other hand, comparison between the predicted elastic modulus and elastic-plastic behaviors of the samples with their corresponding experimental data revealed that the random orientation in conjunction with hollow structural form gives the best results. Moreover, the selected material model for the thermoplastic elastomer i.e., isotropic hardening can precisely describe the mechanical behavior in both tension and compression modes. It is also concluded that the main source of error in this modeling methodology can be attributed to the effects of interface between polymer and nanotubes and orientation in perpendicular directions.

Keywords

Iranian Journal of Polymer Science and Technology
Volume 27, Issue 5 - Serial Number 5
November and December 2014
Pages 421-409

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